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Research Article
Shape evolution and collective excitations in 190Hg: A study using IBM1 and IBM2 models
expand article infoAlyaa A. Abd-Aljbar‡, Mahdi J. S. Al Musawi§, Huda H. Kassim|, Asmaa A. Elbndag, Mushtaq A. Al-Jubbori#, I. Hossain¤, Fadhil I. Sharrad|«, N. Aldahan|«
‡ Department of Medical Physics, Al-Karkh University of Science, Baghdad, Iraq
§ Deptartment of Medical Physics, College of Medicine, University of Kerbala, Karbala, Iraq
| Department of Physics, College of Science, University of Kerbala, Karbala, Iraq
¶ Department of Physics, Faculty of Science, University of Tripoli, Tripoli, Libya
# Departments of Physics, College of Education for Pure Sciences, University of Mosul, Mosul, Iraq
¤ Department of Physics, Rabigh College of Science & Arts, King Abdulaziz University, Rabigh, Saudi Arabia
« College of Health and Medical Technology, University of Alkafeel, Najaf, Iraq
Open Access

Abstract

The Interacting Boson Models, IBM1 and IBM2, analyzed in their O(6) limit are used to describe the properties of the 190Hg isotope. A fitting procedure is used to determine the most accurate parameters to the calculated energy levels of this nucleus. The calculated ground, gamma, and beta bands energy of each model are compared to the previously measured data. Quadrupole electromagnetic transition strengths for 190Hg, obtained from both IBM1 and IBM2, are presented and associated with previously experimental results. Finally, potential energy surfaces (PES) of 190Hg in the dynamical symmetry O(6) of the IBM1 as an occupation of the restriction of the deformation are determined and discussed. All calculations are satisfied with experimental data.

Keywords

IBM1, IBM2, energy level, beta B(E2), potential energy, 190Hg

Introduction

Iachello and Arima (Iachello and Arima 1987) proposed a new model for collective properties of the mid-mass nuclei, the Interacting Boson Model (IBM1), or more specifically, IBM1. In IBM1, the protons and neutrons were treated as bosons which were identical. IBM2 (Arima et al. 1977; Otsuka et al. 1978) adds a further distinction of bosons based on the type of nucleon they were based on outside the closed shells. Each boson could have either of two angular momentum states, the s - boson (L = 0) and the d - boson (L = 2). In the case of even-even nuclei, IBM1 calls for a conserved number of bosons, N. The model also reproduces three limiting symmetries, which were gamma-soft O(6), vibrational U(5) and rotational SU(3) within U(6) algebra (Long et al. 1995; Iachello 2001). Several authors have proposed the existence of intermediate transitional regions of nuclei, namely, U(5)-O(6), U(5)- SU(3), and SU(3)-O(6) (Casten and McCutchan 2007; Cejnar et al. 2010).

It is not really understood yet, why the shape coexistence and quadruple collectivity at low energies in the neutron mid-shell nuclei around the Z = 82 and N = 126 shell closures were observed. Analytical descriptions of the nuclear structure at critically point of phase transitions have attracted considerable interest during the past decades. The 190Hg nucleus has 80 protons and 110 neutrons (Arima et al. 1977). Its configuration can be expressed in terms of π(h11/2)2 and υ(i13/2)16, i.e. two proton holes and sixteen neutron holes with respect to the double magic nucleus 208Pb. Because every nucleon interacts with every other nucleon, complex numerical methods have to be used to do the diagonalisation of the transitional Hamiltonian in these systems. Some of these configurations permit E2 transitions from yrast excited states to ground state. The nuclear structure evolution by the even-neutron deficient isotope 190Hg has not been well reported in the literature. Studies of various classes of bands and B(E2) values in even-mass mercury isotopes (A = 190) were presented in Refs. (Garcia-Ramos and Heyde 2018; Siciliano et al. 2020; Prassa and Karakatsanis 2021). Lifetime measurements of coexistence in neutron deficient 188Hg were made by Siciliano et al. 2020. Triaxial deformation-Energy surfaces showing coexistence were determined for 195Hg Prassa and Karakatsanis 2021. Garcia-Ramos and Heyde 2018 used the IBM, including configuration mixing, to explain even-even isotopes of mercury in particular, and noted the relationship between the nuclear shape and shape-coherence phenomena.

Recently, application of the IBM1 and the IBM2 models of dynamical symmetry SU(3) to the 158Gd nucleus (Fahmi et al. 2023) has recently been explored. Hossain et al. 2023 investigated the O(6) limit in the 108–112 Ru nuclei on the basis of IBM1 calculations. Energy level properties of the neutron-rich Er-OS nuclei with N = 100, 102 and 104 which were the valence nucleons of double magic nucleus 208Pb nucleus was examined by Al Jubbori et al. 2018, 2020, 2022. Furthermore, more papers have studied the nuclear structure of Hg isotopes and near region by using different techniques (Hossain et al. 2014; Ahmad et al. 2021; Jameel-Un et al. 2022, 2023).

At the moment we are doing 190Hg, as this is in the region between the proton shell closure at Z = 82 and the neutron shell closure at N = 126. The goal of the present manuscript is to apply the IBM1 and IBM2 models to analyses three kind of band structures, the potential energy surface and the B(E2) transition strengths of 190Hg. It is assumed that this nucleus has a gamma-soft O(6) symmetry. Our systematic approach aims at relating the phenomenological interacting boson model, both IBM1 and IBM2, to the experimental data on a three energy bands, a reduced B(E2) transition strengths and the PESs of 190Hg. These comparative studies of the 190Hg nucleus based on an IBM1 and IBM2 model are reported here for the first time.

Calculation technique

Interacting Boson Model-1 (IBM1)

Two or more nuclei that have the same number of protons and different numbers of neutrons are referred to as isotopes. The model space for the IBM model is restricted to a smaller space. It gives a mathematical description of unpaired by coupling them in pairs, L = 0 or L = 2. The Hamiltonian for IBM1 is given in references (Iachello and Arima 1987; Casten and Warner 1988).

H=εs(s†⋅s~)+εd(d†⋅d~)

+∑L=0,2,42L+12CL[[(d†×d†](L)×[d~×d~](L)](0)

+12v2[[d†×d†](2)×[d~×s~](2)+[d†×s†](2)×[d~×d~](2)](0)

+12v0[[d†×d†](0)×[s~×s~](0)+[s†×s†](0)×[d~×d~](0)](0)

+12u0[[s†×s†](0)×[s~×s~](0)](0)+u2[[d†×s†](2)×[d~×s~](2)](0) (1)

The Hamiltonian of the IBM1 model is made up of nine terms. Two of them correspond to one body contributions (L = 0 and L = 2), and the parameters εs and εd are the energies of s- and d- bosons, and the others are two body interactions for which the coefficients (C0, C1, C4, v0, v2, u0, u2) are written. The N, the number of bosons, is a conserved quantity. In total, the Hamiltonian for the IBM1 is in Eq. 1 (Arima and Iachello 1976, 1978):

H^=εn^d+a0P^⋅P^+a1L^⋅L^+a2Q^⋅Q^+a3T^3⋅T^3+a4T^4⋅T^4 (2)

Boson energy ε = εd – εs, and the operators are as follows:

n^d=d†⋅d~

P^=0.5[(d~⋅d~)−(s~⋅s~)]

L^=10[d†×d~](1)

Q^=[d†×s~+s†×d~](2)+χ[d†×d~](2)

T^r=[d†×d~](r) (3)

The four operators are indicated by the symbols n̂d, P̂, L̂, Q̂ where, n̂d (total amount of d – bosons) P̂ (pairing), L̂ (angular momentum), and Q̂ (quadruple) operator. The T̂r denotes hexadecapole and octupole operator for r = 4 and 3. The representation χ denotes to the quadrupole creation limits 0 and ±√7/2 (Iachello 1980). The symbol a0, a1, a2, a3 and a4 are limits for the designate the P̂, L̂, Q̂, and T̂r connections between the bosons.

The IBM1 makes three sorts of active symmetry and eigenvalues are given by equation 4 (Iachello 1980).

E(nd,v,L)=εnd+a112nd(nd+4)+(a37−a110−3a470)v(v+3)+114(a4−a3)L(L+1),U(5)

E(λ,μ,L)=a22(λ2+μ2+λμ+3(λ+μ))+(a1−2a28)L(L+1),

E(σ,τ,L)=a04(N−σ)(N+σ+4)+a32τ(τ+3)+(a1−a310)(L(L+1) (4)

The symbol ε, a0, and a2 indicate to the limits for U(5), O(6), and SU(3), respectively. The Hamiltonian (Arima and Iachello 1976; Iachello and Arima 1987) is familiar for the designs that break rendering to equations 5:

H^=a0P^⋅P^+a1L^⋅L^+a2Q^⋅Q^ (5)

Interacting Boson Model-2 (IBM2)

IBM2 (Arima et al. 1977; Otsuka et al. 1978) is a variant of the interacting-boson model that considers the nucleus to consist of protons and neutrons, provides for the differentiation of the two kinds of bosons, and counts their number for which the nucleons are outside the major closed shells. Each boson has a nonzero value of the angular momentum, L = 0 or L = 2, and therefore can exist in one of two states, the s-boson (L = 0) or the d-boson (L = 2). In the case of nuclei whose protons number and neutrons number is even, these bosons that represent protons and neutrons are grouped into collective states with L = 0 and L = 2. The symbol s and d represent these values of angular momentum. Bosons of protons and neutrons are denoted by p and n, respectively; therefore, sπ and sυ are protons and neutrons s bosons (L = 0), and dπ and dv are protons, and neutrons d bosons (L = 2).

In IBM2, the equation (6) gives Hamiltonian as:

H=Hv+Hπ+Vπv (6)

where Hπ and Hv are the Hamiltonians of proton and neutron boson, while Vπv is the interaction of proton-neutron.

A basic Hamiltonian (Puddu et al. 1980):

H=ε(n^dπ+n^dv)+kQπ⋅Qv+Vππ+Vvv+Mπv (7)

Where εv, επ are the neutron and proton energies, respectively, assumed that (εv = επ = ε), and the quadrupole operator is

Qρ=(d†×s+s†×d~)ρ2+χρ(d†×d~)ρ2ρ=π,v (8)

where χp is a parameter to calculate the structure of the boson quadruple operators. The relations Vππ + Vvv suggest d – bosons preserving residual n-n and p-p interactions. We can get equation (9).

V^ρρ=∑k=1.2412(2L+1)12CLρ[(dρ†×dρ†)(L)⋅(d~ρ×d~ρ)(L)](0) (9)

The last term, Majorana interactions Mπv, is written as equation (10).

Mπv=ξ2(sv†×dπ†−dv†×sπ†)2⋅(sv×dπ†−dv†×sπ)2−2∑k=1,3ξk(dv†×dπ†)(k)⋅(d~v×d~π)(k) (10)

If there is investigational confirmation for mixed symmetry states formerly the Majorana parameters are diverse to fix the site of these states in the spectrum. The energy level are calculated using computer code NPBOS (Otsuka and Yoshida 1985). We diagonalizable Hamiltonian of equation (7) and agree the parameters ε, k, xπ, xv and CL for the best acceptable measured data.

Consequences and argument

R4/2 classifications for symmetry

The collective energies of even-even nuclei are consists of three groups based on the ratio R4/2:

R4/2=E(41+)E(21+) (11)

where E(41+) the energy level at 41+ and E(21+) is the energy level at 21+. Even-even nuclei can be classified according to ratios R4/2 (Klein 1980; Singh and Chen 2020; NNDC 2026). The R4/2 = 2.00 indicate a harmonic vibrator U(5), R4/2 = 2.50 indicates g-unstable O(6) symmetry and R4/2 = 3.33 indicate an axially symmetric rotor SU(3)(Iachello and Arima 1987). We recognized O(6) symmetry for 190Hg nucleus since R4/2 values of nucleus is 2.5 (Singh and Chen 2020; NNDC 2026) presented in Table 1. The ratio of E(41+)/ E(21+) values as a function of even neutron numbers of 190Hg isotope is shown in Fig. 1. The solid line shows U(5), O(6) and SU(3) symmetry (Iachello and Arima 1987). The solid line O(6) is near to the data ratios of R4/2 values of 190Hg isotope (Iachello and Arima 1987; Klein 1980; Singh and Chen 2020; NNDC 2026).

Figure 1. 

E(4)/ E(2) Vs even number of neutron of 190Hg isotope. Solid line represented by error indicate U(5), O(6) and SU(3) limit.

Table 1.

The ratio R4/2 = E41+ / E21+ for even-even 190Hg nucleus

Nucleus 190Hg
EXP. 2.50
IBM1 2.45
IBM2 2.456

Boson number

A boson, e.g., s(L = 0) or d(L = 2) boson, describes a pair of valence nucleons, i.e., a proton and a neutron. The boson number is determined by counting the number of pairs, of course the valence nucleons together. Valence nucleons are worked out with the help of double - mirror nuclei. In the present study, valence nucleons are counted with respect to the doubly magic nucleus 208Pb (Z = 82, N = 126). The number of valence protons Np and valence neutrons Nn would give a total boson number N = Np+Nn/2 bosons. For this purpose, 208Pb is considered an inert core for the boson counting. For 190Hg nucleus, the number of valence protons and neutrons are 2 and 16, respectively. Thus the total boson number for 190Hg is (2/2+ 16/2) = 9 as in Table 2.

Table 2.

The parameters used for IBM1 calculations for 190Hg isotope. These parameters unit are in MeV, Furthermore, N and CHQ (χ) without unit

Nucleus N π + Nn = N ε a0 a1 a2 a3 a4 CHQ (χ)
190Hg 1 + 8 = 9 0.000 0.1279 0.0179 0.000 0.2203 0.000 0.000

Energy levels in 190Hg

We have analyzed the excitation spectra of the ground-band, gamma-band and beta band of the 190Hg isotope. In both of IBM models within O(6) limit energy levels of the g-, gamma and beta band was calculated. The energy ratio R = E41+ / E21+ is taken as an indicator of nuclear symmetry. For 190Hg, a level ratio R = 2.50 (Singh and Chen 2020; NNDC 2026) is measured which points to a deformed, gamma soft O(6) symmetry (Iachello and Arima 1987).

Tables 2, 3 shows parameters used in the calculation of IBM1 and IBM2 for the 190Hg isotope, respectively. In Table 2, all the parameters are expressed in MeV and consist of the expected N and CHQ(x) for the case of IBM1. In Table 3, the parameters are also given in MeV for IBM2. Table 4 contains comparative study of ground state band, gamma-band and beta-band of 190Hg nucleus. The calculated data from IBM1 and 2 are in good agreement with earlier experimental measurements. Fig. 2 presents a systematic comparison of the three types of bands, which were calculated with IBM1, IBM2 and with the formerly measured data for the 190Hg nucleus. The results of the calculations of the g - band in the 190Hg nucleus with IBM1 and IBM2 are in satisfy to the measured data. The precision of the calculations in the IBM2 band is higher than the precision of the calculations in the IBM1 band.

Figure 2. 

Comparison of g-band, g-band and b-band of 190Hg nucleus by IBM1, IBM2 and previous measured data (Klein 1980; Singh and Chen 2020; NNDC 2026).

Table 3.

The parameters used for IBM2 calculations for 190Hg isotope. These parameters unit are in MeV

Nucleus N π + Nn = N εd kπv cπ cn x 2 C0Lπ C0Lv(χ)
190Hg 1 + 8 = 9 0.660 -0.095 -1.120 -1.300 -0.001 -0.600 0.000 0.007 -0.100 0.100 0.00
Table 4.

Comparative study of g-band, g-band and b-band in 190Hg isotope by IBM1 and IBM2

g-band g-band b-band
Jπ IBM1 IBM2 EXP Jπ IBM1 IBM2 EXP Jπ IBM1 IBM2 EXP
01+ 0.000 0.000 0.000 22+ 1.076 1.016 1.099 02+ 1.280 0.923 1.278
21+ 0.416 0.416 0.416 31+ 1.932 1.481 1.657 23+ 1.696 1.461 1.558
41+ 1.020 1.022 1.041 42+ 1.900 1.719 1.850* 43+ 2.300 2.280 2.342*
61+ 1.812 1.624 1.772 51+ 2.960 2.158 –
81+ 2.792 2.334 2.573* 62+ 2.912 2.365 2.509

Electric Reduced Transition Probabilities B(E2)

The energy levels of excited states of even-even nuclei are given as Li+ = 21+, 41+, 61+, 81+.......) generally decay to the lower-lying state Lf+ = Li+-2 through E2 transition. Study of strength of the reduced transition probability B(E2) is one of very important parameter to under the decay properties of a nucleus. At present work the B(E2) data were calculated using the computer code PHINT (Scholten 1991), which requires values for effective charge (eB) from Eq. (12).

B(E2:21+→01+)=α225N(N+4)=eB25N(N+4) (12)

In order to obtain reduced transition probability values, we have close-fitting the calculated absolute strengths B(E2) of transitions within ground state band to experimental ones. Value of effective charge (a2) of IBMI has been determined by normalizing experimental data B(E2;21+ → 01+) of isotope using Eq. (12). The value of parameter a22 for isotope has been calculated from the given measured value of transitions (21+ → 01+) and used to calculate B(E2) values for transitions 41+ → 21+, 61+ → 41+ and 81+ → 61+.The model wave functions were found by diagonalization of the IBM2 Hamiltonian and the program NPBEM (Otsuka and Yoshida 1985) were used to estimate the electromagnetic transition.

The E2 transition operator (Lange et al. 1982):

T(E2)=eπQπ+evQv (13)

Where, Qρ is the quadrupole operator and has the same definition as in Hamiltonian (7). ℮π and ℮v are boson effective charges contingent on the boson number N and they can be obtained by fitting B(E2;21+ → 01+) to the measured data. The effective charge a in e.b and eb in e.b and B(E2) value in e2b2 by IBM1, IBM2 and previous experimental data is presented in Table 5. The B(E2) data of IBM1 and IBM2 are consistent with the measured data. The reduced transition probability B(E2) is a microscopic interpretation of nuclear structure.

Table 5.

Reduced transition probability B(E2)↓ in even-even 190Hg nucleus, (e π = 0.167, e ν = 0.184) in the IBM2

Nucleus a e.b Transition level B(E2) exp. e2.b2 B(E2) IBM1 e2.b2 B(E2) IBM2 e2.b2
190Hg 0.1117 21+ → 01+ 0.2921 0.2920 0.2650
22+ → 01+ – 0.0409 0.0139
41+ → 21+ 0.2596 0.3990 0.4351
42+ → 21+ – 0.0320 0.0130
42+ → 22+ – 0.2287 0.1580
61+ → 41+ 0.0419 0.4367 0.4201
81+ → 61+ – 0.4356 0.5146

Potential Energy Surface (PES)

The potential energy surface (PES) gives good indication to the infinitesimal and symmetric shapes of nuclei. IBM Hamiltonian in the Refs (Bentley and Frauendorf 2011; Nomura et al. 2011; Kassim et al. 2020; Waheed et al. 2020) is used to create the PES plots using the Skyrme mean-field method. For IBM1, the energy surface is given as the expectation value of the IBM1 Hamiltonian (eq. 1) in the coherent state |N, ꞵ, γ⟩ (Siciliano et al. 2020). The creation operators bc† act on the boson vacuum |0⟩ in order to create this coherent state as follows:

"N,β,γ⟩=1N!(bc†)N"0⟩ (14)

where

bc†=11+β2{s†+β[cos⁡γ(do†)+1/2sin⁡γ(d2†+d−2†)]} (15)

then, the PES can be written in terms of β and γ as:

E(N,β,γ)=Nεdβ2(1+β2)+N(N+1)(1+β2)2[α1β4+α2β3cos⁡3γ+α3β2+α4] (16)

Alpha’s parameters are the coefficients CL, v2, vo and uo in Eq. (1). The factor (attribute) of beta is related to the total deformation of the nucleus. A nucleus can be sphere shaped or distorted depending on whether the value of beta is equal to zero or not. Additionally, the term gamma describes the symmetry of the nucleus, i.e., when gamma = 0, the nucleus is prolate and when gamma = 60 deg, the nucleus is oblate. Fig. 3 shows the PES contour plot for 190Hg. The PES values in MeV are indicated on the color panel.

Figure 3. 

The PES contour plot for 190Hg nucleus.

Conclusions

In the IBM1 and the IBM2 models, we examined the three types of bands ground, Gamma, and beta, the reduced transition strength B E2 as well as the potential energy surface of 190Hg. The calculated data from IBM1 and 2 are in good agreement with earlier experimental measurements. The values of the B(E2) predicted by both of these IBM calculations, IBM1 and IBM2, are consistent with the existing measurements. Potential energy surface of 190Hg is studied with IBM1. All calculations for 190Hg with IBM1 and IBM2 are limited within the O(6) limit.

Acknowledgements

We are grateful to the University of Alkafeel for their assistance with this research work. We thank Prof. Dr. Akram J. Karim, Brunel University, UK, for editing the English language.

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Conflict of interest

The authors have declared that no competing interests exist.

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Author contributions

Alyaa A. Abd-Aljbar contributed to the research concept, manuscript writing and manuscript formatting. Mahdi J. S. Al Musawi contributed to the literature review and data organization. Huda H. Kassim contributed to the theoretical calculations and data interpretation. Asmaa A. Elbndag contributed to the data analysis, preparation of figures and tables. Mushtaq A. Al-Jubbori contributed to the methodology and scientific review of the manuscript. I. Hossain contributed to the validation of results and proofreading. Fadhil I. Sharrad supervised the research, contributed to the interpretation of results, and revised the manuscript. N. Aldahan contributed to data checking and final manuscript review. All authors have read and approved the final version of the manuscript.

Data availability

All of the data that support the findings of this study are available in the main text.

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